7–11 Jul 2025
University of the Witwatersrand, Johannesburg
Africa/Johannesburg timezone

Magnetic behavior of Ar implanted ZnO

Not scheduled
20m
Solomon Mahlangu House (University of the Witwatersrand, Johannesburg)

Solomon Mahlangu House

University of the Witwatersrand, Johannesburg

Poster Presentation Track A - Physics of Condensed Matter and Materials Poster Session

Speaker

Vusumuzi Masondo (Durban University of Technology)

Description

Our research is driven by the goal to realize ferromagnetism at room temperature on non-magnetic materials such as semiconductors, among other materials. If realized, semiconductor functionality should coexist with ferromagnetism, ideally above room temperature (practical operating temperatures). In our work, ZnO single crystals implanted with 45 keV 40Ar ions up to fluences of 4.5×1015 ions/cm2 were selected as a system of interest. Emission Mössbauer Spectroscopy (eMS) measurements were then carried out on the samples following implantation with 57Mn* radioactive ion beams, which decay to the Mössbauer atom 57Fe via β- decay. Radioactive ion beams were produced at the ISOLDE facility, at CERN, through a fission reaction induced by 1.4 GeV protons on a UC2 target, followed by a multi-stage laser ionization and mass separation by pure magnets. Two sets of measurements were carried out: (a) Temperature series measurements on the as-implanted sample and on another Ar implanted ZnO sample following annealing at 400 0C in vacuum for 15 minutes, and (b) Angle dependence measurements on the annealed sample, in the presence of an external magnetic field. Temperature dependence measurements show strong magnetic features in the spectrum, with the magnetic field not dependent on the temperature, thus paramagnetism instead of ferromagnetism. Paramagnetism is further confirmed by the angle dependence of magnetic sextet lines in each spectrum. A comparison and discussion of results obtained will be presented.

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Primary author

Vusumuzi Masondo (Durban University of Technology)

Co-authors

Prof. Krish Bharuth-Ram (Durban University of Technology) Prof. Carsten Ronning (University of Jena) Dr Hilary Masenda (University of the Witwatersrand) Dr Heraldur Gunnlaugsson (University of Iceland) Ms Ongeziwe Mpatani (University of the Witwatersrand) Dr Lehlohonolo Lisema (University of the Witwatersrand) Dr Sanele Dlamini (Durban University of Technology) Dr Torben Molholt (DTU Health Technology) Prof. Deena Naidoo (University of the Witwatersrand) Dr Juliana Heiniger-Schell (CERN) Dr Bingcui Qi (University of Iceland) Dr Petko Krastev (Institute for Nuclear Research and Nuclear Energy) Dr Sveinn Olafsson (University of Iceland)

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